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Experimental signatures of phase interference and subfemtosecond time dynamics on the incident energy axis of resonant inelastic x-ray scattering

Author(s): Wray, L. Andrew; Huang, Shih-Wen; Xia, Yuqi; Hasan, M. Zahid; Mathy, Charles; et al

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dc.contributor.authorWray, L. Andrew-
dc.contributor.authorHuang, Shih-Wen-
dc.contributor.authorXia, Yuqi-
dc.contributor.authorHasan, M. Zahid-
dc.contributor.authorMathy, Charles-
dc.contributor.authorEisaki, Hiroshi-
dc.contributor.authorHussain, Zahid-
dc.contributor.authorChuang, Yi-De-
dc.date.accessioned2019-08-29T17:07:02Z-
dc.date.available2019-08-29T17:07:02Z-
dc.date.issued2015-01en_US
dc.identifier.citationWray, L Andrew, Huang, Shih-Wen, Xia, Yuqi, Hasan, M. Zahid, Mathy, Charles, Eisaki, Hiroshi, Hussain, Zahid, Chuang, Yi-De. (2015). Experimental signatures of phase interference and subfemtosecond time dynamics on the incident energy axis of resonant inelastic x-ray scattering. Physical Review B, 91 (3), 10.1103/PhysRevB.91.035131en_US
dc.identifier.issn1098-0121-
dc.identifier.urihttp://arks.princeton.edu/ark:/88435/pr1c720-
dc.description.abstractCore hole resonance is used in X-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic X-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators SrCuO2 and NiO to examine how resonance states decay into different excitation symmetries at the transition metal M-, L- and K-edges. Quantum interference patterns characteristic of the two major RIXS mechanisms are identified within the data, and used to distinguish the attosecond scale scattering dynamics by which fundamental excitations of a many-body system are created. A function is proposed to experimentally evaluate whether a particular excitation has constructive or destructive interference in the RIXS cross-section, and corroborates other evidence that an anomalous excitation is present at the leading edge of the Mott gap in quasi-one dimensional SrCuO2.en_US
dc.format.extent1 - 12en_US
dc.language.isoen_USen_US
dc.relation.ispartofPhysical Review Ben_US
dc.rightsAuthor's manuscripten_US
dc.titleExperimental signatures of phase interference and subfemtosecond time dynamics on the incident energy axis of resonant inelastic x-ray scatteringen_US
dc.typeJournal Articleen_US
dc.identifier.doidoi:10.1103/PhysRevB.91.035131-
dc.date.eissued2015-01-27en_US
dc.identifier.eissn1550-235X-
pu.type.symplectichttp://www.symplectic.co.uk/publications/atom-terms/1.0/journal-articleen_US

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